Functionalized biochars with highly-efficient malachite green adsorption property produced from banana peels via microwave-assisted pyrolysis
文献类型: 外文期刊
作者: Chen, Long 1 ; Mi, Baobin 1 ; He, Jiangnan 1 ; Li, Yuchen 1 ; Zhou, Zhi 1 ; Wu, Fangfang 1 ;
作者机构: 1.Hunan Agr Univ, Coll Agron, Coll Biosci & Biotechnol, Hunan Engn Res Ctr Biochar,Sch Chem & Mat Sci, Changsha 410128, Hunan, Peoples R China
2.Hunan Acad Agr Sci, Res Inst Vegetables, Changsha 410125, Peoples R China
关键词: Microwave-assisted pyrolysis; Functionalized biochar; Graphite-like structure; Malachite green; Adsorption mechanism
期刊名称:BIORESOURCE TECHNOLOGY ( 影响因子:11.4; 五年影响因子:10.6 )
ISSN: 0960-8524
年卷期: 2023 年 376 卷
页码:
收录情况: SCI
摘要: In this study, functionalized banana peel biochar (BPB) was prepared by microwave-assisted pyrolysis for the first time to investigate its adsorption to malachite green (MG) dye. Adsorption experiments showed that the maximum adsorption capacity of BPB500 and BPB900 to malachite green reached 1790.30 and 2297.83 mg.g(-1) within 120 min. The adsorption behaviour was well-fitted by the pseudo-second-order kinetic model and Langmuir isotherm model, and Delta G(0) < 0, Delta H-0 > 0, indicated that the adsorption process was endothermic and spontaneous, dominated by chemisorption. The adsorption mechanism of MG dye on BPB included hydrophobic interaction, hydrogen bonding, pi-pi interaction, n-pi interaction, and ion exchange. Meanwhile, through regeneration tests, simulated wastewater treatment experiments, and cost calculations, it was found that BPB has great potential for practical applications. This work demonstrated that microwave-assisted pyrolysis is a viable low-cost approach for producing excellent sorbents from biomass, and banana peel is a promising feedstock to prepare biochar for dye removal.
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